CO2 Corrosion Resistance in Packer Elements

CO2 Corrosion Resistance in Packer Elements: Detailed Findings and Engineering Recommendations

Packer elements are crucial in maintaining well integrity in gas wells, providing reliable seals under extreme conditions. However, CO2 corrosion poses a significant threat to these elements, especially under compressive stress. A recent comprehensive study has given us valuable insights into the performance of hydrogenated nitrile butadiene rubber (HNBR) and nitrile rubber (NBR) in such environments. Here, we summarize the study’s findings and offer recommendations for engineers in the selection and maintenance of packer elements for gas wells.

Materials Used

  1. HNBR (Hydrogenated Nitrile Butadiene Rubber):
    • Known for its excellent heat, oil, and chemical resistance, making it a preferred choice for harsh environments.
  2. NBR (Nitrile Butadiene Rubber):
    • Commonly used due to its good resistance to oils and fuels, but generally less resistant to high temperatures and chemicals compared to HNBR.

Greater Reactivity in Liquid CO2

Rubber samples exposed to liquid CO2 showed significantly greater degradation than those exposed to gaseous CO2. This was evident through increased weight change, reduced hardness, and higher compression set values. For instance, HNBR samples exposed to liquid CO2 showed a weight change rate of up to 0.28%, compared to 0.071% in gaseous CO2.

Impact of Compressive Stress

Compressive stress exacerbated the corrosion effects of CO2 on both HNBR and NBR. Under compressive loads ranging from 0 to 12 kN, both types of rubber showed increased degradation in mechanical properties, with liquid CO2 causing more severe damage than gaseous CO2. The study revealed that higher loads led to more significant material degradation.

Weight Change and Hardness Reduction

After CO2 exposure, the weight of rubber samples increased, indicating material absorption and swelling. For example, NBR samples showed weight change rates from 0.015% to 0.28%, depending on the phase of CO2 and the applied load. Hardness reduction was more pronounced in liquid CO2, with HNBR samples showing a decrease from an initial hardness of approximately 90 Shore A to as low as 58 Shore A after exposure under high load conditions.

Compression Set Increase

Compression set, which measures the permanent deformation of rubber after compression, increased significantly after exposure to CO2. For HNBR samples, compression set values ranged from 10.59% to 22.40% in liquid CO2, compared to 7.04% to 11.08% in the control group.

Microstructural Damage

SEM analysis showed that rubber samples exposed to liquid CO2 exhibited severe structural damage, such as holes and fractures, particularly under higher compressive loads. This microstructural damage correlates with the observed deterioration in mechanical properties.

Elemental Composition Changes

EDS analysis indicated significant changes in the elemental composition of the rubber materials after CO2 exposure. For instance, the carbon content in HNBR decreased from 67.58% to 57.87% in liquid CO2, reflecting the material’s chemical interaction with CO2.

Engineering Recommendations

Based on these findings, engineers should consider the following recommendations when selecting and maintaining packer elements for gas wells:

Material Selection

  1. Prefer HNBR Over NBR:
    • Given its superior performance in CO2 environments, HNBR should be prioritized for packer elements. Its resistance to high temperatures, oils, and chemicals makes it more suitable for harsh well conditions.
  2. Use Peroxide-Cured Compounds:
    • Peroxide curing agents enhance the thermal stability and chemical resistance of rubber materials. Selecting peroxide-cured HNBR compounds can provide better performance under high temperature, high pressure (HTHP) conditions.

Preventive Measures

  1. Regular Monitoring:
    • Implement regular inspection and monitoring of packer elements to detect early signs of degradation. Use non-destructive testing methods such as ultrasound or radiography to identify internal flaws and material deterioration without removing the packer from the well.
  2. Environmental Control:
    • Minimize CO2 exposure by using gas dehydration and inhibitor injection techniques. Controlling the environment can significantly reduce the rate of CO2-induced corrosion.

Design Considerations

  1. Account for Compressive Stress:
    • Ensure that the design of packer elements accounts for the additional stress caused by compression. Use materials and designs that can withstand both chemical and mechanical stresses. For example, designing thicker rubber elements or incorporating metal reinforcements can help mitigate the effects of compressive stress.
  2. Protective Coatings:
    • Apply protective coatings to rubber elements to provide an additional barrier against CO2 corrosion. These coatings should be designed to withstand high temperatures and pressures, further enhancing the durability of the packer elements.

Maintenance Strategies

  1. Preventive Replacement:
    • Plan for preventive replacement of packer elements based on the operational conditions and expected service life. This proactive approach can prevent unexpected failures and reduce downtime, ensuring continuous well operation.
  2. Use of Additives:
    • Incorporate antioxidants and other specialty additives in the rubber compounds to enhance corrosion resistance and extend the service life of packer elements. Additives like carbon black and silica can improve the mechanical properties and resistance of rubber to corrosive environments.

Conclusion

The study highlights the critical impact of CO2 corrosion on HNBR and NBR materials used in packer elements under compressive stress. By selecting the right materials, implementing preventive measures, and considering environmental control, engineers can significantly improve the reliability and performance of packer elements in gas wells. Adopting these detailed recommendations will help mitigate the risks associated with CO2 corrosion, ensuring safer and more efficient gas well operations.

References

Zhu, D., Lin, Y., Ma, H., Zhang, H., Li, Y., Zhang, L. and Deng, K., 2017. Experimental studies on CO2 corrosion of rubber materials for packer under compressive stress in gas wells. Engineering Failure Analysis, 80, pp.11-23.